A General Approach to the Basiliolide/Transtaganolide Natural Products: Total Syntheses of Basiliolide B, epi‐8‐Basiliolide B, Transtaganolide C, and Transtaganolide D
Identifieur interne : 000050 ( Main/Exploration ); précédent : 000049; suivant : 000051A General Approach to the Basiliolide/Transtaganolide Natural Products: Total Syntheses of Basiliolide B, epi‐8‐Basiliolide B, Transtaganolide C, and Transtaganolide D
Auteurs : Hosea M. Nelson [États-Unis] ; Kei Murakami [États-Unis] ; Virgil [États-Unis] ; Stoltz [États-Unis]Source :
- Angewandte Chemie International Edition [ 1433-7851 ] ; 2011-04-11.
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Abstract
In a flash: The total synthesis of transtaganolide and basiliolide natural products is achieved in three steps from achiral, monocyclic esters (see scheme). Featured in the syntheses are an Ireland‐Claisen/Diels–Alder cascade and a novel methoxyacetylide coupling/cyclization sequence.
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DOI: 10.1002/anie.201008003
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